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1-Bromobenzocyclobutene

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CAS:21120-91-2
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Products Intro: Product Name: 1-Bromobenzocyclobutene
CAS: 21120-91-2
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1-Bromobenzocyclobutene Basic information
Product Name:1-Bromobenzocyclobutene
Synonyms:1-BROMOBENZOCYCLOBUTENE;1-BroMobenzocyclobutene;7-BroMobicyclo[4.2.0]octa-1,3,5,7-tetraene;1-BrBCB 1-Bromobenzocyclobutene;1-Bromobenzocyclobutene 95%;Bicyclo[4.2.0]octa-1,3,5-triene, 7-bromo-;1-Bromobenzocyclobutene ISO 9001:2015 REACH;1-bromo-1,2-dihydrobenzocyclobutene
CAS:21120-91-2
MF:C8H7Br
MW:183.05
EINECS:
Product Categories:Aluminium foil bag/Fluoride bottle or on your request;API intermediates;Alkenyl;Halogenated Hydrocarbons;Organic Building Blocks
Mol File:21120-91-2.mol
1-Bromobenzocyclobutene Structure
1-Bromobenzocyclobutene Chemical Properties
Boiling point 90 °C/10.5 mmHg (lit.)
density 1.45 g/mL at 25 °C (lit.)
refractive index n20/D 1.59(lit.)
Fp 205 °F
storage temp. Sealed in dry,Room Temperature
AppearanceColorless to light yellow Liquid
InChIInChI=1S/C8H7Br/c9-8-5-6-3-1-2-4-7(6)8/h1-4,8H,5H2
InChIKeyJQOFZAWKFBCSHK-UHFFFAOYSA-N
SMILESC12C(C(Br)C1)=CC=CC=2
Safety Information
WGK Germany 3
HS Code 2903898090
Storage Class10 - Combustible liquids
MSDS Information
ProviderLanguage
SigmaAldrich English
1-Bromobenzocyclobutene Usage And Synthesis
Chemical PropertiesColorless to pale yellow liquid
Uses1-Bromobenzocyclobutene may be used in the synthesis of following compounds:
  • five-membered zirconacycles
  • benzocyclobutenol and benzocyclobutenone
  • 2,3-dimethoxyprotoberberinium bromide, via reaction with 3,4-dihydro-6,7-dimethoxyisoquinoline
Application1-Bromobenzocyclobutene is a halogenated aromatic fine chemical intermediate that can be used in drug development, semiconductor materials, and organic synthesis.
General Description1-Bromobenzocyclobutene is a useful synthon. It has important applications in organometallic methodology. Reaction between cycloheptatriene, bromoform, potassium carbonate and 18-crown-6 at 140°C yields 1-bromobenzocyclobutene.
Synthesis
Bromoform

75-25-2

Cycloheptatriene

544-25-2

1-Bromobenzocyclobutene

21120-91-2

In a 250 mL round bottom flask equipped with a drying tube and condenser, cycloheptatriene (30.7 g, 300 mmol), tribromomethane (25.3 g, 100 mmol), anhydrous K2CO3 (15.0 g, 109 mmol), and 18-crown-6 (0.75 g) were added. The mixture was heated with stirring at 145°C for 9-10 hours. After completion of the reaction, the solution was allowed to cool to room temperature and diluted with an equal volume of acetone. Silica gel (15.0 g) was added to the reaction mixture and the insoluble solid residue was separated by vacuum filtration and the filter cake was washed with acetone until the washings were colorless. The filtrate was concentrated and the residual cycloheptatriene was removed by distillation. The viscous brown residue was dissolved in hot petroleum ether and the filtrate was concentrated after removing the precipitate by filtration. Vacuum distillation through a Vigreaux column gave slightly impure 1-bromobenzocyclobutene. Further purification by redistillation gave pure 1-bromobenzocyclobutene (2.95 g, 5.94% yield) as a light yellow liquid.1H NMR (300 MHz, CDCl3) δ 7.28 (m, 1H, ArH), 7.16 (d, 1H, J = 7.0 Hz, ArH), 7.07 (d, 1H, J = 6.4 Hz, ArH), 7.07 (d, 1H, J = 6.4 Hz, ArH) 5.39 (m, 1H, CH), 3.85 (dd, 1H, J = 4.4 Hz, J = 14.7 Hz, CH2), 3.45 (d, 1H, J = 14.7 Hz, CH2).

References[1] Patent: WO2008/24435, 2008, A2. Location in patent: Page/Page column 104
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